The solution is shown below.
Enter the angle of the change difference in AddRotate. This time, I’m only tilting Pitch by 1.
FRotator Rotate = PoseableMeshComponent->GetBoneRotationByName(BoneName,EBoneSpaces::Type::WorldSpace);
FRotator AddRotate = FRotator(1,0,0);
FRotator NewRotate = FRotator(FQuat(AddRotate) * FQuat(Rotate));
PoseableMeshComponent->SetBoneRotationByName(BoneName,NewRotate,EBoneSpaces::Type::WorldSpace);